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Rotational diffusion model with a variable collision distribution

Creator

Elsken, J. van der;

Wegdam, G.H.;

Frenkel, D.

Publisher

American institute of physics

Date

1972

Description

Starting with an m-diffusion model a matrix description is given of the rotational motion of a dipole molecule undergoing frequent collisions. This treatment gives rise to an analytical expression for the dipole correlation function and for the angular momentum correlation function in which a limited number of parameters from the model appear. It is argued that the collision distribution which determines the rotational diffusion process need not necessarily be a Poisson distribution. In liquids with strong interactions the distribution is governed by the frequency distribution of the medium. This leads to the inclusion of a librational motion in the rotational diffusion model. A comparison of simulations with different collision distributions and experimental data is given

Subject

Geneeskunde

Type

Article

Format

image/pdf

Identifier

Journal of chemical physics 57(7), 2691-2697 (1972)

http://igitur-archive.library.uu.nl/chem/2006-0504-200021/UUindex.html

Database

DSpace at Utrecht University

Language

Rights

Elsken, J. van der

Wegdam, G.H.

Frenkel, D.

info:eu-repo/semantics/openAccess

Link to record

http://retrievo.keep.pt/record?id=oai:dspace.library.uu.nl:1874/8750

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Downloaded 11 Oct 2004 to 145.18.129.130. Redistribution subject to AIP license or copyright, see http://jcp.aip.org/jcp/copyright.jsp

Downloaded 11 Oct 2004 to 145.18.129.130. Redistribution subject to AIP license or copyright, see http://jcp.aip.org/jcp/copyright.jsp

Downloaded 11 Oct 2004 to 145.18.129.130. Redistribution subject to AIP license or copyright, see http://jcp.aip.org/jcp/copyright.jsp

Downloaded 11 Oct 2004 to 145.18.129.130. Redistribution subject to AIP license or copyright, see http://jcp.aip.org/jcp/copyright.jsp

Downloaded 11 Oct 2004 to 145.18.129.130. Redistribution subject to AIP license or copyright, see http://jcp.aip.org/jcp/copyright.jsp

Downloaded 11 Oct 2004 to 145.18.129.130. Redistribution subject to AIP license or copyright, see http://jcp.aip.org/jcp/copyright.jsp

Downloaded 11 Oct 2004 to 145.18.129.130. Redistribution subject to AIP license or copyright, see http://jcp.aip.org/jcp/copyright.jsp

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Rotational diffusion model with a variable collision distribution

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